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Letters written to Gay from political and literary contemporaries such as Horace Greeley, Charles Sumner, and William Bryant; reports in letter form from his reporters at the front during the Civil War; and personal correspondence including many letters from his wife, Elizabeth Neall Gay. Letters written to Mrs. Gay from family friends and business associates including many from her husband. Correspondence of other members of the Gay family including Walter Gay, Sarah Gay, and Allan Gay. Diaries, notebooks, and journals of Sydney Howard Gay.

Correspondence and papers of various members of the Kane and Hand families. The collection includes the business correspondence of Oliver Kane of Albany (early 19th century); the correspondence of Moses Hand (1764-1826) of Baltimore; the letters and papers of Thomas Jennings Hand (1824-1908) of New York, with many letters from Professor William Hand Browne of John Hopkins; the diaries and account books of Thomas Jennings Hand, extending from 1859 to 1901, and the household account books of his wife; the family correspondence, accounts, and personal papers of Oliver Kane-Hand (1863-1941); various legal documents and papers of Oliver Kane-Hand (1863-1941); various legal documents and papers of Oliver Kane King, Thomas Jennings Hand, Jr. and Oliver Kane-Hand; and a group of family photographs.